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1.
Opt Express ; 32(6): 10563-10576, 2024 Mar 11.
Artigo em Inglês | MEDLINE | ID: mdl-38571264

RESUMO

Fresnel incoherent correlation holography (FINCH) enables high-resolution 3D imaging of objects from several 2D holograms under incoherent light and has many attractive applications in motionless 3D fluorescence imaging. However, FINCH has difficulty implementing 3D imaging of dynamic scenes since multiple phase-shifting holograms need to be recorded for removing the bias term and twin image in the reconstructed scene, which requires the object to remain static during this progress. Here, we propose a dual-channel Fresnel noncoherent compressive holography method. First, a pair of holograms with π phase shifts obtained in a single shot are used for removing the bias term noise. Then, a physic-driven compressive sensing (CS) algorithm is used to achieve twin-image-free reconstruction. In addition, we analyze the reconstruction effect and suitability of the CS algorithm and two-step phase-shift filtering algorithm for objects with different complexities. The experimental results show that the proposed method can record hologram videos of 3D dynamic objects and scenes without sacrificing the imaging field of view or resolution. Moreover, the system refocuses images at arbitrary depth positions via computation, hence providing a new method for fast high-throughput incoherent 3D imaging.

2.
Opt Express ; 31(19): 30932-30946, 2023 Sep 11.
Artigo em Inglês | MEDLINE | ID: mdl-37710625

RESUMO

In this paper, we investigate the singular multi-wavelength and multi-waveband transparencies generated by P T-symmetric dumbbell optical waveguide networks composed of two materials, and obtain the number regularity for the transparency wavelengths of one-unit-cell system and the general relationships for the transmission and reflection coefficients of multi-unit-cell systems. Consequently, three types of exact transparencies produced by multi-unit-cell systems are found based on the aforementioned formulas: (i)exact multi-wavelength unidirectional or bidirectional transparency as the same as those of one-unit-cell system; (ii)exact multi-wavelength bidirectional transparency at which one-unit-cell system cannot produce exact transparency, generated by adjusting the number of unit cells; (iii)exact multi-wavelength bidirectional transparency at which one-unit-cell system produces exact transparency, also generated by adjusting the number of unit cells. It provides theoretical foundations for developing highly sensitive and multi-wavelength optical filters. On the other hand, we also discover that multi-unit-cell systems can create approximate multi-waveband bidirectional transparencies by adjusting the number of unit cells, which provides scientific support for developing high-performance optical stealth devices.

3.
Anal Chem ; 95(36): 13614-13619, 2023 Sep 12.
Artigo em Inglês | MEDLINE | ID: mdl-37639529

RESUMO

9-Mesityl-10-methylacridinium ion (Acr+-Mes) is a donor-acceptor molecule with a much longer lifetime and a higher energy electron transfer excited state than natural photosynthetic reaction centers. Unlike lucigenin with a coplanar geometry, Acr+-Mes has an orthogonal geometry. There is no π conjugation between Acr+ and Mes. Due to its special electron donor-acceptor structure, it does not rely on strong alkalinity to generate an electron transfer state like lucigenin, which makes it possible to achieve chemiluminescence (CL) under weakly alkaline or neutral conditions. In this study, we report Acr+-Mes CL for the first time. Acr+-Mes generates about 400 times stronger CL intensity than lucigenin under neutral conditions (pH = 7) using KHSO5 as the coreactant. Moreover, Co2+ can enhance Acr+-Mes/KHSO5 CL remarkably. Acr+-Mes/KHSO5 CL enables Co2+ detection with a linear range of 0.5-500 nM and a limit of detection of 28 pM (S/N = 3). This method was tested for the detection of Co2+ in lake water, and the standard recovery rate of 96.8-107% was achieved. This study provides a new way to develop efficient CL systems in neutral solutions.

4.
Anal Chem ; 95(24): 9380-9387, 2023 06 20.
Artigo em Inglês | MEDLINE | ID: mdl-37285116

RESUMO

Metal-organic gels (MOGs) are a category of metal-organic smart soft materials with large specific surface areas, loose porous structures, and open metal active sites. In this work, trimetallic Fe(III)Co(II)Ni(II)-based MOGs (FeCoNi-MOGs) were synthesized at room temperature via a simple and mild one-step procedure. Fe3+, Co2+, and Ni2+ were the three central metal ions in it, while 1,3,5-benzenetricarboxylic acid (H3BTC) served as the ligand. The solvent enclosed in it was then removed by freeze-drying to get the corresponding metal-organic xerogels (MOXs). The as-prepared FeCoNi-MOXs have excellent peroxidase-like activity and can significantly enhance luminol/H2O2 chemiluminescence (CL) by more than 3000 times, which is very effective compared with other reported MOXs. Based on the inhibitory effect of dopamine on the CL of the FeCoNi-MOXs/luminol/H2O2 system, a simple, rapid, sensitive, and selective CL method for dopamine detection was established with a linear range of 5-1000 nM and a limit of detection of 2.9 nM (LOD, S/N = 3). Furthermore, it has been effectively used for the quantitative measurement of dopamine in dopamine injections and human serum samples, with a recovery rate of 99.5-109.1%. This research brings up prospects for the application of MOXs with peroxidase-like activity in CL.


Assuntos
Dopamina , Luminol , Humanos , Luminol/química , Peróxido de Hidrogênio/química , Luminescência , Metais/química , Peroxidases , Medições Luminescentes/métodos , Limite de Detecção
6.
Opt Express ; 31(10): 16192-16204, 2023 May 08.
Artigo em Inglês | MEDLINE | ID: mdl-37157703

RESUMO

The perfect optical vortex (POV) beam carrying orbital angular momentum with topological charge-independent radial intensity distribution possesses ubiquitous applications in optical communication, particle manipulation, and quantum optics. But the mode distribution of conventional POV beam is relatively single, limiting the modulation of the particles. Here, we originally introduce the high-order cross-phase (HOCP) and ellipticity γ into the POV beam and construct all-dielectric geometric metasurfaces to generate irregular polygonal perfect optical vortex (IPPOV) beams following the trend of miniaturization and integration of optical systems. By controlling the order of the HOCP, conversion rate u, and ellipticity factor γ, various shapes of IPPOV beams with different electric field intensity distributions can be realized. In addition, we analyze the propagation characteristics of IPPOV beams in free-space, and the number and rotation direction of bright spots at the focal plane give the magnitude and sign of the topological charge carried by the beam. The method does not require cumbersome devices or complex calculation process, and provides a simple and effective method for simultaneous polygon shaping and topological charge measurement. This work further improves the beam manipulation ability while maintaining the characteristics of the POV beam, enriches the mode distribution of the POV beam, and provides more possibilities for particle manipulation.

7.
Nanomaterials (Basel) ; 13(10)2023 May 14.
Artigo em Inglês | MEDLINE | ID: mdl-37242054

RESUMO

Multichannel metasurfaces are becoming a significant trend in the field of optical encryption due to their excellent manipulation of optical wavefronts. However, existent multichannel metasurfaces for optical encryption mostly implement only two channels in the near-field, or three channels by combining the near- and far-field. In this paper, we propose and simulate a three-channel metasurface that works entirely in the near-field and uses the polarization state of the incident light, left circularly polarized (LCP) light, right circularly polarized (RCP) light, and linearly polarized (LP) light as the security key. The metasurface consists of two types of nanostructures that work as a polarizer and a quarter-wave plate, providing an additional degree of freedom for encoding that enables independent near-field display at 633 nm wavelength incident light. The proposed three-channel metasurface has the advantages of high information density and high security, which will pave the way for multi-channel applications such as ultracompact displays, optical encryption, and information storage.

8.
Nanomaterials (Basel) ; 13(6)2023 Mar 17.
Artigo em Inglês | MEDLINE | ID: mdl-36985988

RESUMO

Integrating multiple independent functions into a single optical component is one of the most important topics in research on photoelectric systems. In this paper, we propose a multifunctional all-dielectric metasurface that can achieve a variety of non-diffractive beams depending on the polarization state of the incident light. Using the anisotropic TiO2 rectangular column as the unit structure, the three functions of generating polygonal Bessel vortex beams under left-handed circularly polarized incidence, Airy vortex beams under right-handed circularly polarized incidence and polygonal Airy vortex-like beams under linearly polarized incidence are realized. In addition, the number of polygonal beam sides and the position of focal plane can be adjusted. The device could facilitate further developments in scaling complex integrated optical systems and fabricating efficient multifunctional components.

9.
Opt Express ; 30(26): 47338-47349, 2022 Dec 19.
Artigo em Inglês | MEDLINE | ID: mdl-36558664

RESUMO

The resonant optical tunneling effect (ROTE) originates from the frustrated total reflection effect because unique transmission characteristics are used to study high-sensitivity sensors. In this study, we theoretically demonstrated that choosing a suitable transmission gap made it possible for the ROTE structure based on hexagonal boron nitride and graphene to obtain a large Goos-Hänchen shift as high as tens of thousands of times the incident wavelength at a specific incident angle. The amplitude of the Goos-Hänchen shift was found to be sensitive to the central layer thickness but was also modulated by the tunneling gap on both sides. In addition, adjusting the chemical potential and relaxation time of the graphene sheets could alter the Goos-Hänchen shift. Our work provides a new way to explore the Goos-Hänchen effect and opens the possibility for the application of high-precision measurement technology based on the ROTE.

10.
Nanomaterials (Basel) ; 12(19)2022 Oct 06.
Artigo em Inglês | MEDLINE | ID: mdl-36234620

RESUMO

A novel one-dimensional parity-time-symmetric periodic ring optical waveguide network (1D PTSPROWN) is constructed using magnesium fluoride (MgF2), by adjusting the length ratio of gain and loss materials in PT-symmetric waveguide and ordinary dielectric material, and by optimizing the program to search for the extremum spontaneous PT-symmetric breaking points. The ultra-strong transmission, reflection, and photonic location are noticed in the proposed 1DPTSPROWN as compared with the other PT-symmetric optical waveguide networks. The maximum and minimum reached 1018 and 10-15, respectively, which is more than 6 orders of magnitude greater and 3 orders of magnitude smaller than the best results reported so far. The ultra-strong transmission and reflection peaks, ultra-weak transmission, and reflection valleys generated by electromagnetic waves in this network were found to have interesting resonance and anti-resonance effects. Furthermore, frequency of periodic cycles and violet or redshift laws were discovered in the 1D PTSPROWN of fixed length ratio of gain and loss material in the PT-symmetric waveguide by adjusting the ratio of the upper and lower arm lengths of waveguides. The proposed optical waveguide network might have potential application in the design of CPA lasers, high-efficiency optical accumulators, and several other devices.

11.
Opt Express ; 30(10): 17541-17553, 2022 May 09.
Artigo em Inglês | MEDLINE | ID: mdl-36221574

RESUMO

Achromatic metalens have the potential to significantly reduce the size and complexity of broadband imaging systems. A large variety of achromatic metalens has been proposed and most of them have the fixed achromatic band that cannot be actively modified. However, band-tunable is an important function in practical applications such as fluorescence microscopic imaging and optical detection. Here, we propose a bilayer metalens that can switch achromatic bands by taking the advantage of the high refractive index contrast of Sb2S3 between amorphous and crystalline state. By switching the state of Sb2S3, the achromatic band can be reversibly switched between the red region of visible spectrum (650-830 nm) and the near-infrared spectrum (830-1100 nm). This band-tunable design indicates a novel (to our knowledge) method to solve the problem of achromatic focusing in an ultrabroad band. The metalens have an average focusing efficiency of over 35% and 55% in two bands while maintaining diffraction-limited performance. Moreover, through proper design, we can combine different functionalities in two bands such as combining achromatic focusing and diffractive focusing. The proposed metalens have numerous potential applications in tunable displaying, detecting devices and multifunctional devices.

12.
Opt Express ; 30(11): 18434-18446, 2022 May 23.
Artigo em Inglês | MEDLINE | ID: mdl-36221644

RESUMO

The operation of near-field and far-field can be employed to display holographic and nanoprinting images, which significantly improves the information density. Previous studies have proposed some approaches to display the images independently or simultaneously, but cannot satisfy these two characteristics in a single structure under the same incident light. Here, a single layer multifunctional metasurface is proposed to display a nanoprinting image and a holographic image independently and simultaneously. By tailoring the dimensions of each nanobricks and adopting different orientation angle, the amplitude and phase can be artificially designed. Moreover, enabled by the simulated annealing algorithm, we take the impact of both amplitude and phase of each nanobrick into consideration, which eliminates the unnecessary influence of amplitude on holographic image. Compared with previous work, our metasurfaces markedly improve the quality of holographic image with simple structures while not affecting the nanoprinting image. To be exact, it breaks the coupling between the near-field and far-field, achieving independent and simultaneous control of both fields. Our proposed metasurfaces carry characteristics of simple manufacture, little crosstalk, and great compactness, which provides novel applications for image displays, optical storage and information technology.

13.
Opt Express ; 30(21): 37888-37898, 2022 Oct 10.
Artigo em Inglês | MEDLINE | ID: mdl-36258368

RESUMO

In this study, a one-dimensional (1D) two-material period ring optical waveguide network (TMPROWN) was designed, and its optical properties were investigated. The key characteristics observed in the 1D TMPROWN include the following: (1) Bound states in continuum (BICs) can be generated in the optical waveguide network. (2) In contrast to the BICs previously reported in optical structures, the range of the BICs generated by the 1D TMPROWN is not only larger, but also continuous. This feature makes it possible for us to further study the electromagnetic wave characteristics in the range of the BICs. In addition, we analyzed the physical mechanisms of the BICs generated in the 1D TMPROWN. The 1D TMPROWN is simple in structure, demonstrates flexibility with respect to adjusting the frequency band of the BICs, and offers easy measurement of the amplitude and phase of electromagnetic waves. Hence, further research on high-power super luminescent diodes, optical switches, efficient photonic energy storage, and other optical devices based on the 1D TMPROWN designed in this study is likely to have implications in a broad range of applications.

14.
Opt Express ; 30(17): 30303-30311, 2022 Aug 15.
Artigo em Inglês | MEDLINE | ID: mdl-36242137

RESUMO

A rational number harmonic mode-locked dual-loop optoelectronic oscillator (RHML-DL-OEO) is proposed and experimentally demonstrated. In the proposed system, an external radio frequency (RF) signal and a feedback oscillating microwave signal drive two arms of a dual-drive Mach-Zehnder modulator (DMZM). Mode locking is realized by frequency detuning. The larger effective free spectrum range (FSR) and higher side-mode suppression result from the Vernier effect effectively suppress supermode noise and intermodulation distortions (IMDs). Experimental results demonstrate that the microwave frequency comb (MFC) signals with repetition frequencies of 901.8 kHz, 2.3046 MHz and 5.3106 MHz are generated by 9th-, 23rd- and 53rd-order rational number harmonic mode-locking, respectively. Compared with the rational number harmonic mode-locked optoelectronic oscillator based on single-loop structure, the supermode noise suppression ratios of the scheme we propose are improved by 30.5 dB, 27.6 dB and 20.3 dB, respectively. Furthermore, the performance of single sideband (SSB) phase noise is also investigated.

15.
Opt Express ; 30(17): 30881-30893, 2022 Aug 15.
Artigo em Inglês | MEDLINE | ID: mdl-36242184

RESUMO

The perfect vortex (PV) beam, characterized by carrying orbital angular momentum and a radial electric intensity distribution independent of the topological charge, has important applications in optical communication, particle manipulation, and quantum optics. Conventional methods of generating PV beams require a series of bulky optical elements that are tightly collimated with each other, adding to the complexity of optical systems. Here, making the amplitude of transmitted co-polarized and cross-polarized components to be constant, all-dielectric transmission metasurfaces with superimposed phase profiles integrating spiral phase plate, axicon and Fourier lens are constructed based on the phase-only modulation method. Using mathematical derivation and numerical simulation, multi-channel PV beams with controllable annular ring radius and topological charge are realized for the first time under circularly polarized light incidence combining the propagation phase and geometric phase. Meanwhile, perfect vector vortex beams are produced by superposition of PV beams under the incidence of left-handed circularly polarized and right-handed circularly polarized lights, respectively. This work provides a new perspective on generating tailored PV beams, increasing design flexibility and facilitating the construction of compact, integrated, and versatile nanophotonics platforms.

16.
Sci Rep ; 12(1): 14887, 2022 09 01.
Artigo em Inglês | MEDLINE | ID: mdl-36050471

RESUMO

The use of low-dose aspirin in older adults is increasing as is the prevalence of osteoporosis. Aspirin has been shown in numerous studies to affect bone metabolism. However, there is no clear link between low-dose aspirin use and bone mineral density (BMD). This study examined differences in bone mineral density between low-dose aspirin users and non-aspirin users in adults aged 50-80 years. We conducted a cross-sectional study of 15,560 participants who participated in the National Health and Nutrition Examination Survey (NHANES) 2017-March 2020. We used a multivariate logistic regression model to evaluate the relationship between low-dose aspirin and femoral neck BMD, femoral total BMD, intertrochanteric BMD, and the first lumbar vertebra BMD (L1 BMD) in patients aged 50 to 80 years. A total of 1208 (Group 1: femoral neck BMD, total femur BMD, and intertrochanter BMD) and 1228 (Group 2: L1 BMD) adults were included in this study. In both group 1 and group 2, BMD was higher in the low-dose aspirin group than in the non-aspirin group (Total femur BMD ß = 0.019, 95% CI 0.004-0.034; Femoral neck BMD ß = 0.017, 95% CI 0.002-0.032; Intertrochanter BMD ß = 0.025, 95% CI 0.007-0.043; L1 BMD ß = 0.026, 95% CI 0.006-0.046). In subgroup analyses stratified by gender, this positive association existed in both gender after adjusting for confounders. On subgroup analyses stratified by age, this positive association existed in three different age groups after adjusting for confounders. To test whether the effect of low-dose aspirin on BMD was affected by gender and age, the interaction P value was greater than 0.05. These findings from a human study looking into the relationship between low-dose aspirin use and BMD suggest that regular low-dose aspirin may be associated with a higher BMD. The association between low-dose aspirin and BMD did not differ by age group or gender.


Assuntos
Densidade Óssea , Colo do Fêmur , Absorciometria de Fóton , Idoso , Aspirina/efeitos adversos , Estudos Transversais , Colo do Fêmur/diagnóstico por imagem , Humanos , Vértebras Lombares/diagnóstico por imagem , Inquéritos Nutricionais
17.
Opt Express ; 30(9): 13994-14001, 2022 Apr 25.
Artigo em Inglês | MEDLINE | ID: mdl-35473153

RESUMO

A novel photonic-assisted method for radio frequency (RF) signal amplification with high-gain and narrowband based on a dual-loop optoelectronic oscillator (OEO) is proposed and experimentally demonstrated. In the proposed system, the low-power RF signal is injected into a dual-loop OEO which is below the threshold oscillation state. And the maximum gain is obtained when the frequency of the RF signal matches with the potential oscillation mode of the dual-loop OEO. The approach provides an average gain greater than 22 dB for the RF signal which matches with oscillation mode. After amplification, the signal-to-noise ratio (SNR) turns out to be 40 dB. Furthermore, the 3 dB bandwidth of the suggested system can be narrower than 1.2 kHz which can effectively remove the out-of-band noise and spurious effects. Meanwhile, the performance of sensitivity and phase noise are also investigated.

18.
Opt Express ; 30(9): 14146-14160, 2022 Apr 25.
Artigo em Inglês | MEDLINE | ID: mdl-35473165

RESUMO

The Talbot-like effect of symmetric Pearcey beams (SPBs) is presented numerically and experimentally in the free space. Owing to the Talbot-like effect, the SPBs have the property of periodic, multiple autofocusing and self-healing. Meanwhile, the focusing positions and focusing times of SPBs are controlled by the beam shift factor and the distribution factors. Furthermore, the beam shift factor can also affect the Talbot-like effect and the Talbot period. It is believed that the results can diversify the application of the Talbot effect.

19.
Anal Chem ; 94(18): 6853-6859, 2022 05 10.
Artigo em Inglês | MEDLINE | ID: mdl-35476395

RESUMO

The ability to estimate and quantify biothiols in biological fluids is very significant for attaining a detailed understanding of biothiols-related pathological diseases. Most of the developed methods for biothiols detection are not suitable for this purpose owing to their low sensitivity, poor selectivity, and long experimental procedures. In this study, a novel and simple structure electrochemical probe has been synthesized for the first time for the selective determination of biothiols. The developed probe is based on using 2,4-dinitrobenzenesulfonyl moiety (DNBS) as a selective recognition moiety for biothiols. The electrochemical probe was successfully fabricated through a facile one-step reaction between 2,4-dinitrobenzenesulfonyl chloride (DNBS-Cl) and p-aminophenol. The successful synthesis of the probe was confirmed by using different characterization techniques such as an NMR spectroscopy, Fourier-transform infrared (FT-IR) spectroscopy, and mass spectrometry. Biothiols can selectively cleave the DNBS moiety through an aromatic nucleophilic substitution (ANS) reaction within 10 min to release p-aminophenol, which is a highly electrochemical active molecule that can be selectively detected easily by cyclic voltammetry at low potential. The probe has been employed for the quantification of cysteine, glutathione, and homocysteine with a LOD of 1.50, 3.48, and 4.67 µM, respectively. Excellent recoveries have been achieved in the range of 95.44-98.71% for the determination of the total biothiols in the human plasma sample.


Assuntos
Cisteína , Corantes Fluorescentes , Cisteína/química , Corantes Fluorescentes/química , Glutationa/análise , Homocisteína , Humanos , Espectrometria de Fluorescência , Espectroscopia de Infravermelho com Transformada de Fourier , Compostos de Sulfidrila/análise
20.
Nanomaterials (Basel) ; 12(7)2022 Apr 06.
Artigo em Inglês | MEDLINE | ID: mdl-35407345

RESUMO

A depolarizer, a kind of optical element that converts polarized light to unpolarized light, has been found massive applications in classical optics. However, depolarizers based on metasurface which can be applied in integrated optics have rarely been proposed. In this paper, an electronically controlled metasurface depolarizer is demonstrated based on the time-domain integral average method and nano-material barium titanate. It obtains emergent light with a degree of polarization reduced to 2.5% when hit by linearly polarized light at 633 nm, and has a transmission efficiency greater than 72%. This depolarizing metasurface can be designed on-demand, immunizing the degree of the emergent light from its size, and has the simple electronic control with high-speed response.

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